After determining the volume of the bounding box, I calculated the required amounts of both parts of the mold solution to mix for my mold. A few minutes of vigorous mixing later, I had a solution that was ready to be degassed.
We placed the solution in the vacuum to properly evacuate any lurking air bubbles in the solution. This took a couple passes but eventually the gas seemed to have been mostly gone from the mold mixture.
After the solution was properly degassed, I carefully poured the mix into my foam-core/clay model, checking for leaks or spills and limiting the amount of air bubbles that popped up.
Since the mold had a 40 minute cure time, it was time to leave and let the solution work its magic!
After a couple days, we came back and cracked open the foam-core box to see our first mold part. After clearing away the clay and some silicone residue, this is what we were left with.